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Citation Details
Title:
Dual-bed catalytic system for the selective reduction of NOx with propene
Category(s):
Non-Ammonia/Urea SCR
Author(s):
J.A. Moulijn
Javier Perez-Rami
Antonio R. Vaccaro
Freek Kapteijn
Journal:
Chemical Engineering and Technology
Publisher:
Wiley-VCH Verlag GmbH, Weinheim, Ger
Year:
2000
Pages:
721-725
Volume:
23
Abstract:
For the removal of NOx from exhausts containing excess oxygen, the selective catalytic reduction of NOx using hydrocarbons (HC-SCR) is highly interesting, especially for car applications (lean deNOx). Two types of HC-SCR catalysts can be distinguished. High-temperature catalysts operate at temperatures above 573 K, showing moderate activity, and (mostly) low heat and poison resistance, but high N2 selectivity. Low-temperature catalysts, usually based on Pt, operate between 473 and 573 K, showing opposite features: very high activity, as well as heat and poison resistance, and a low N2 selectivity by forming N2O. Our strategy for developing an active and stable deNOx system without N2O emission is the implementation of a separate catalytic function for N2O removal as a second stage.
Times Viewed:
1185
Submitter Details
Name:
Vitaly Prikhodko
Email:
prikhodkovy@ornl
Organization:
Oak Ridge National Laboratory
Date Submitted:
2002-10-08

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